A mother singing to her baby...the babies reaction is priceless. Music has a way of moving us all. Watch the eyes ..the expressions on this babies face.
http://screen.yahoo.com/popular/babys-emotional-reaction-mothers-song-144913027.html
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Maybe something about the combination of notes sounds like crying to the baby. Babies start crying when other babies cry, so I think this is like an empathy response to thinking the mother is crying. Maybe a happier sounding song is better to sing around babies for the development of musical abilities without upsetting the baby.